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External electric field manipulations on structural phase transition of vanadium dioxide nanoparticles and its application in field effect transistor
Li, W. W.1; Zhu, J. J.1; Liang, J. R.2,4; Hu, Z. G.1; Liu, J.1,3; Chen, H. D.2; Chu, J. H.1
刊名Journal of physical chemistry c
2011-12-01
卷号115期号:47页码:23558-23563
ISSN号1932-7447
DOI10.1021/jp207196g
通讯作者Hu, z. g.(zghu@ee.ecnu.edu.cn)
英文摘要Despite the intensive study on the famous metal insulator transition, many questions regarding the evolution of the structural phase transition (spt) in vanadium dioxide (vo(2)) remain unresolved. here, the lattice vibrations and spt of vo(2) nanoparticles on a sio(2)/si(100) substrate with different applied voltage from 0 to 8 v have been investigated by raman scattering spectra. it can be found that both the intensities of the a(g) and b(g) phonon modes decrease with increasing temperature. moreover, the vibration modes disappear when heating up to the temperature of spt (t(spt)). with the voltage increasing from 0 to 8 v, the t(spt) decreases from 68.3 to 64.3 degrees c for the heating process and from 66.3 to 58.8 degrees c for the cooling process, respectively. the fitting results reveal that the t(spt) was decreased by -0.48 and -0.87 degrees c/v in the heating and cooling processes, respectively. this is because the larger electric field could assist the shortening of the v-v distance and the change of carriers between electrons and the mixing of electrons and holes. moreover, the t(spt) delay was increased by 0.4 degrees c/v with increasing the positive voltage because the electric field can pull the electrons and push the holes. the present results of the vo(2) three-terminal device show a potential realization of the vo(2)-based field effect transistor.
WOS关键词METAL-INSULATOR-TRANSITION ; CRYSTALLINE VO2 NANOBEAMS ; THIN-FILMS ; OPTICAL-PROPERTIES ; MOTT TRANSITION ; NANOSTRUCTURES ; ORGANIZATION ; DOMAINS ; DEVICES
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
WOS类目Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000297195200037
内容类型期刊论文
URI标识http://www.corc.org.cn/handle/1471x/2428357
专题半导体研究所
通讯作者Hu, Z. G.
作者单位1.E China Normal Univ, Dept Elect Engn, Minist Educ, Key Lab Polar Mat & Devices, Shanghai 200241, Peoples R China
2.Chinese Acad Sci, Inst Semicond, State Key Lab Integrated Optoelect, Beijing 100083, Peoples R China
3.Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China
4.Tianjin Univ, Sch Elect & Informat Engn, Tianjin 300072, Peoples R China
推荐引用方式
GB/T 7714
Li, W. W.,Zhu, J. J.,Liang, J. R.,et al. External electric field manipulations on structural phase transition of vanadium dioxide nanoparticles and its application in field effect transistor[J]. Journal of physical chemistry c,2011,115(47):23558-23563.
APA Li, W. W..,Zhu, J. J..,Liang, J. R..,Hu, Z. G..,Liu, J..,...&Chu, J. H..(2011).External electric field manipulations on structural phase transition of vanadium dioxide nanoparticles and its application in field effect transistor.Journal of physical chemistry c,115(47),23558-23563.
MLA Li, W. W.,et al."External electric field manipulations on structural phase transition of vanadium dioxide nanoparticles and its application in field effect transistor".Journal of physical chemistry c 115.47(2011):23558-23563.
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