Fractionation, distribution and transport of mercury in rivers and tributaries around wanshan hg mining district, guizhou province, southwestern china: part 2-methylmercury | |
Zhang, Hua1,2; Feng, Xinbin1; Larssen, Thorjorn3,4; Shang, Lihai1; Vogt, Rolf D.4; Lin, Yan4; Li, Ping1; Zhang, Hui1,2 | |
刊名 | Applied geochemistry
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2010-05-01 | |
卷号 | 25期号:5页码:642-649 |
ISSN号 | 0883-2927 |
DOI | 10.1016/j.apgeochem.2010.01.005 |
通讯作者 | Feng, xinbin(fengxinbin@vip.skleg.cn) |
英文摘要 | Water samples were collected during normal flow (2007) and during a drought period (2008) from five rivers and tributaries draining the wanshan hg mining district, guizhou, china. unfiltered methylmercury (mehg) as well as particulate and dissolved fractions of mehg (p-mehg, d-mehg) were measured to assess the spatial and temporal variation of mehg contamination in the local river system. most locations (about 80%) displayed higher mehg concentrations during drought period than during normal discharge conditions. concentrations of mehg during the drought period ranged from <0.035 to 11 ng l(-1) (geometric mean: 0.43), while during normal flow the concentrations ranged from <0.035 to only 3.4 ng l(-1) (geometric mean: 0.21). concentrations of mehg were positively correlated with total hg (thg) concentrations (r(2) = 0.20-0.58, p < 0.001) and inversely related to distance from the calcines, during both sampling periods (r(2) = 0.34 and 0.23, p < 0.001, for low and normal flow, respectively) indicating that calcines may be important sources of mehg to the downstream environment. approximately 39% of mehg was bound to particulates and the rest was transported in the dissolved phase along stretches of the entire river, which was different from thg, as this was mainly transported bound to particulates (commonly more than 80%). (c) 2010 elsevier ltd. all rights reserved. |
WOS关键词 | SURFACE WATERS ; METHYL MERCURY ; MINE WASTES ; FRESH-WATERS ; CARSON RIVER ; METHYLMERCURY ; SPECIATION ; AREAS ; SPECTROSCOPY ; ETHYLATION |
WOS研究方向 | Geochemistry & Geophysics |
WOS类目 | Geochemistry & Geophysics |
语种 | 英语 |
出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
WOS记录号 | WOS:000278674900004 |
内容类型 | 期刊论文 |
URI标识 | http://www.corc.org.cn/handle/1471x/2411961 |
专题 | 中国科学院大学 |
通讯作者 | Feng, Xinbin |
作者单位 | 1.Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550002, Peoples R China 2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China 3.Norwegian Inst Water Res, N-0169 Oslo, Norway 4.Univ Oslo, Dept Chem, N-0315 Oslo, Norway |
推荐引用方式 GB/T 7714 | Zhang, Hua,Feng, Xinbin,Larssen, Thorjorn,et al. Fractionation, distribution and transport of mercury in rivers and tributaries around wanshan hg mining district, guizhou province, southwestern china: part 2-methylmercury[J]. Applied geochemistry,2010,25(5):642-649. |
APA | Zhang, Hua.,Feng, Xinbin.,Larssen, Thorjorn.,Shang, Lihai.,Vogt, Rolf D..,...&Zhang, Hui.(2010).Fractionation, distribution and transport of mercury in rivers and tributaries around wanshan hg mining district, guizhou province, southwestern china: part 2-methylmercury.Applied geochemistry,25(5),642-649. |
MLA | Zhang, Hua,et al."Fractionation, distribution and transport of mercury in rivers and tributaries around wanshan hg mining district, guizhou province, southwestern china: part 2-methylmercury".Applied geochemistry 25.5(2010):642-649. |
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