Ultrafast dynamics of chlorobenzene clusters | |
Liu, Benkang1,2; Wang, Bingxing1,2; Wang, Yanqiu1; Wang, Li1 | |
刊名 | chemical physics letters
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2009-08-06 | |
卷号 | 477期号:4-6页码:266-270 |
通讯作者 | 王利 |
产权排序 | 1;1 |
英文摘要 | the ultrafast dynamics of chlorobenzene clusters upon 271 nm excitation is studied by femtosecond pump-probe time-of-flight mass spectrometry. transient profiles of clusters are fitted by two-exponential decay component models, an ultrafast component and a slow decay component. the ultrafast (similar to 170 fs) decay of s(1) state is tentatively attributed to the internal conversion to the high vibrational levels of s(0) state. lifetimes of this ultrafast component decease with the cluster size, due to the influence of the solvation effects, while lifetimes of the slow decay component (>1 ns) increase with the cluster size, due to the increase of freedom degrees. (c) 2009 elsevier b. v. all rights reserved. |
WOS标题词 | science & technology ; physical sciences |
类目[WOS] | chemistry, physical ; physics, atomic, molecular & chemical |
研究领域[WOS] | chemistry ; physics |
关键词[WOS] | analyzed threshold ionization ; photodissociation dynamics ; internal-conversion ; water clusters ; benzene dimer ; aryl halides ; state ; spectroscopy ; complexes ; fragment |
收录类别 | SCI |
原文出处 | false |
语种 | 英语 |
WOS记录号 | WOS:000268515200007 |
公开日期 | 2010-11-30 |
内容类型 | 期刊论文 |
源URL | [http://159.226.238.44/handle/321008/101991] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
作者单位 | 1.Acad Sinica, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China 2.Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Liu, Benkang,Wang, Bingxing,Wang, Yanqiu,et al. Ultrafast dynamics of chlorobenzene clusters[J]. chemical physics letters,2009,477(4-6):266-270. |
APA | Liu, Benkang,Wang, Bingxing,Wang, Yanqiu,&Wang, Li.(2009).Ultrafast dynamics of chlorobenzene clusters.chemical physics letters,477(4-6),266-270. |
MLA | Liu, Benkang,et al."Ultrafast dynamics of chlorobenzene clusters".chemical physics letters 477.4-6(2009):266-270. |
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