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	Spatially separated photosystem ii and a silicon photoelectrochemical cell for overall water splitting: a natural-artificial photosynthetic hybrid
	Wang, Wangyin1; Wang, Hong1,2; Zhu, Qingjun2,3; Qin, Wei1; Han, Guangye3; Shen, Jian-Ren3,4; Zong, Xu1; Li, Can1
刊名	Angewandte chemie-international edition
	2016-08-01
卷号	55期号:32页码:9229-9233
关键词	Photocatalysis Photoelectrochemistry Photosystem ii Water splitting Z-scheme
ISSN号	1433-7851
DOI	10.1002/anie.201604091
通讯作者	Zong, xu(xzong@dicp.ac.cn) ; Li, can(canli@dicp.ac.cn)
英文摘要	Integrating natural and artificial photosynthetic platforms is an important approach to developing solar-driven hybrid systems with exceptional function over the individual components. a natural-artificial photosynthetic hybrid platform is formed by wiring photosystem ii (psii) and a platinum-decorated silicon photoelectrochemical (pec) cell in a tandem manner based on a photocatalytic-pec z-scheme design. although the individual components cannot achieve overall water splitting, the hybrid platform demonstrated the capability of unassisted solar-driven overall water splitting. moreover, h-2 and o-2 evolution can be separated in this system, which is ascribed to the functionality afforded by the unconventional z-scheme design. furthermore, the tandem configuration and the spatial separation between psii and artificial components provide more opportunities to develop efficient natural-artificial hybrid photosynthesis systems.
WOS关键词	PHOTO-BIOELECTROCHEMICAL CELLS ; SHUTTLE REDOX MEDIATOR ; VISIBLE-LIGHT ; ELECTRON-TRANSFER ; Z-SCHEME ; OXYGEN ; SOLAR ; PHOTOCATALYSTS ; SYSTEM ; RESOLUTION
WOS研究方向	Chemistry
WOS类目	Chemistry, Multidisciplinary
语种	英语
出版者	WILEY-V C H VERLAG GMBH
WOS记录号	WOS:000383371800017
内容类型	期刊论文
URI标识	http://www.corc.org.cn/handle/1471x/2376206
专题	中国科学院大学
通讯作者	Zong, Xu; Li, Can
作者单位	1.Chinese Acad Sci, Collaborat Innovat Ctr Chem Energy Mat IChEM, Dalian Natl Lab Clean Energy, State Key Lab Catalysis,Dalian Inst Chem Phys, Zhongshan Rd 457, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Chinese Acad Sci, Inst Bot, Key Lab Photobiol, Photosynthesis Res Ctr, Beijing 100093, Peoples R China 4.Okayama Univ, Grad Sch Nat Sci & Technol, Photosynthesis Res Ctr, 1-1 Naka 3 Chome, Okayama 7008530, Japan
推荐引用方式 GB/T 7714	Wang, Wangyin,Wang, Hong,Zhu, Qingjun,et al. Spatially separated photosystem ii and a silicon photoelectrochemical cell for overall water splitting: a natural-artificial photosynthetic hybrid[J]. Angewandte chemie-international edition,2016,55(32):9229-9233.
APA	Wang, Wangyin.,Wang, Hong.,Zhu, Qingjun.,Qin, Wei.,Han, Guangye.,...&Li, Can.(2016).Spatially separated photosystem ii and a silicon photoelectrochemical cell for overall water splitting: a natural-artificial photosynthetic hybrid.Angewandte chemie-international edition,55(32),9229-9233.
MLA	Wang, Wangyin,et al."Spatially separated photosystem ii and a silicon photoelectrochemical cell for overall water splitting: a natural-artificial photosynthetic hybrid".Angewandte chemie-international edition 55.32(2016):9229-9233.

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