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Assessment of global mercury deposition through litterfall
Wang, Xun1,2; Bao, Zhengduo3,4; Lin, Che-Jen1,3,4; Yuan, Wei1,2; Feng, Xinbin1
刊名Environmental science & technology
2016-08-16
卷号50期号:16页码:8548-8557
ISSN号0013-936X
DOI10.1021/acs.est.5b06351
通讯作者Lin, che-jen(jerry.lin@lamar.edu) ; Feng, xinbin(fengxinbin@vip.skleg.cn)
英文摘要There is a large uncertainty in the estimate of global dry deposition of atmospheric mercury (hg). hg deposition through litterfall represents an important input to terrestrial forest ecosystems via cumulative uptake of atmospheric hg (most hg-0) to foliage. in this study, we estimate the quantity of global hg deposition through litterfall using statistical modeling (monte carlo simulation) of published data sets of litterfall biomass production, tree density, and hg concentration in litter samples. on the basis of the model results, the global annual hg deposition through litterfall is estimated to be 1180 +/- 710 mg yr(-1), more than two times greater than the estimate by geos-chem. spatial distribution of hg deposition through litterfall suggests that deposition flux decreases spatially from tropical to temperate and boreal regions. approximately 70% of global hg-0 dry deposition occurs in the tropical and subtropical regions. a major source of uncertainty in this study is the heterogeneous geospatial distribution of available data. more observational data in regions (southeast asia, africa, and south america) where few data sets exist will greatly improve the accuracy of the current estimate. given that the quantity of global hg deposition via litterfall is typically 2-6 times higher than hg-0 evasion from forest floor, global forest ecosystems represent a strong hg-0 sink.
WOS关键词REMOTE UPLAND FOREST ; ACADIA NATIONAL-PARK ; ATMOSPHERIC MERCURY ; DRY DEPOSITION ; SOUTHWESTERN CHINA ; ELEMENTAL MERCURY ; METHYL MERCURY ; ISOTOPE SIGNATURES ; TROPICAL FORESTS ; ATLANTIC FOREST
WOS研究方向Engineering ; Environmental Sciences & Ecology
WOS类目Engineering, Environmental ; Environmental Sciences
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000381654600016
内容类型期刊论文
URI标识http://www.corc.org.cn/handle/1471x/2375113
专题中国科学院大学
通讯作者Lin, Che-Jen; Feng, Xinbin
作者单位1.Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550081, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Lamar Univ, Ctr Adv Water & Air Qual, Beaumont, TX 77710 USA
4.Lamar Univ, Dept Civil & Environm Engn, Beaumont, TX 77710 USA
推荐引用方式
GB/T 7714
Wang, Xun,Bao, Zhengduo,Lin, Che-Jen,et al. Assessment of global mercury deposition through litterfall[J]. Environmental science & technology,2016,50(16):8548-8557.
APA Wang, Xun,Bao, Zhengduo,Lin, Che-Jen,Yuan, Wei,&Feng, Xinbin.(2016).Assessment of global mercury deposition through litterfall.Environmental science & technology,50(16),8548-8557.
MLA Wang, Xun,et al."Assessment of global mercury deposition through litterfall".Environmental science & technology 50.16(2016):8548-8557.
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