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	Self-powered fluorescence display devices based on a fast self-charging/recharging battery (mg/prussian blue)
	Zhang, Hui1,2; Yu, You1,2; Zhang, Lingling1,2; Zhai, Yiwen1,2; Dong, Shaojun1,2
刊名	Chemical science
	2016
卷号	7期号:11页码:6721-6727
ISSN号	2041-6520
DOI	10.1039/c6sc02347a
通讯作者	Dong, shaojun(dongsj@ciac.ac.cn)
英文摘要	Stimuli-responsive (such as voltage and/or light) fluorescence display systems have attracted particular attention in their promising fields of application. however, there are few examples of self-powered fluorescence display devices. here we designed and fabricated a self-powered fluorescence display device based on a fast-charging/recharging battery. the specially designed battery was composed of a prussian blue (pb) cathode and a magnesium metal anode with a high theoretical redox potential difference (similar to 2.8 v). moreover, smartly adding a trace amount of naclo in the electrolyte could realize oxidizing pw to pb similar to 480 times faster than when oxidizing without naclo, leading to the fast self-charging and high power density (maximum power density of 13.34 mw cm(-2), about two to three orders of magnitude larger than previous bio-fuel cells) of the mg/pb battery. most importantly, pb was used as not only the cathodic catalyst but also as an electrochromic material, making it possible to construct a self-powered and rechargeable electrochromic fluorescence display with only two electrodes. besides, fluorescent [ru(bpy)(3)](2+)-doped silica nanoparticles (ru@ sio2), were selected as the fluorescence resonance energy transfer (fret) donor to match pb (fret acceptor). to the best of our knowledge, we demonstrated a self-powered and rechargeable electrochromic fluorescence display with only two electrodes for the first time.
WOS关键词	PRUSSIAN BLUE ; ENERGY-TRANSFER ; PERFORMANCE-CHARACTERISTICS ; COORDINATION POLYMERS ; REVERSIBLE MODULATION ; SILICA NANOPARTICLES ; BIOFUEL CELLS ; ION BATTERY ; ELECTRODES ; NANOWIRES
WOS研究方向	Chemistry
WOS类目	Chemistry, Multidisciplinary
语种	英语
出版者	ROYAL SOC CHEMISTRY
WOS记录号	WOS:000386228900016
内容类型	期刊论文
URI标识	http://www.corc.org.cn/handle/1471x/2375011
专题	中国科学院大学
通讯作者	Dong, Shaojun
作者单位	1.Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Jilin, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式 GB/T 7714	Zhang, Hui,Yu, You,Zhang, Lingling,et al. Self-powered fluorescence display devices based on a fast self-charging/recharging battery (mg/prussian blue)[J]. Chemical science,2016,7(11):6721-6727.
APA	Zhang, Hui,Yu, You,Zhang, Lingling,Zhai, Yiwen,&Dong, Shaojun.(2016).Self-powered fluorescence display devices based on a fast self-charging/recharging battery (mg/prussian blue).Chemical science,7(11),6721-6727.
MLA	Zhang, Hui,et al."Self-powered fluorescence display devices based on a fast self-charging/recharging battery (mg/prussian blue)".Chemical science 7.11(2016):6721-6727.

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