Pattern of atmospheric mercury speciation during episodes of elevated pm2.5 levels in a coastal city in the yangtze river delta, china | |
Hong, Youwei1,2,3,4; Chen, Jinsheng1,2,3; Deng, Junjun1,2,3; Tong, Lei1,2,3; Xu, Lingling1,2,3; Niu, Zhenchuan2; Yin, Liqian1,2,3; Chen, Yanting1,2,3; Hong, Zhenyu1,2,5 | |
刊名 | Environmental pollution |
2016-11-01 | |
卷号 | 218页码:259-268 |
关键词 | Atmospheric mercury Pm2.5 Pollution characteristics Source identification Coastal area |
ISSN号 | 0269-7491 |
DOI | 10.1016/j.envpol.2016.06.073 |
通讯作者 | Chen, jinsheng(jschen@iue.ac.cn) |
英文摘要 | Measurement of atmospheric mercury speciation was conducted in a coastal city of the yangtze river delta, china from july 2013 to january 2014, in conjunction with air pollutants and meteorological parameters. the mean concentrations of gaseous elemental mercury (gem), particulate bound mercury (hgp) and reactive gaseous mercury (rgm) were 3.26 +/- 1.63 ng m(-3), 659 +/- 931 pg m(-3), and 197 246 pg m-3, respectively. high percentages of hgp during haze days were found, due to the increase in direct emissions and gas-particle partitioning of rgm. the average gas-particle partitioning coefficients (kp) during moderate or severe haze days (pm2.5 > 150 mu g m(-3)) were obviously decreased. gem and hgp were positively correlated with pm2.5, so2, no2 and co, suggesting a significant contribution of anthropogenic sources. elevated hgp concentrations in cold seasons and in the morning were observed while rgm exhibited different seasonal and diurnal pattern. the ratio of hgp/so2 and pearson correlation analysis suggested that coal combustion was the main cause of increasing atmospheric hg concentrations. the monitoring site was affected by local, regional and interregional sources. the back trajectory analysis suggested that air mass from northwest china and huabei plain contributed to elevated atmospheric hg in winter and autumn, while southeast china with clean air masses were the major contributor in summer. (c) 2016 elsevier ltd. all rights reserved. |
WOS关键词 | SIZE-FRACTIONATED PARTICLES ; GASEOUS ELEMENTAL MERCURY ; PARTICULATE MERCURY ; REACTIVE MERCURY ; NEW-ENGLAND ; SOURCE APPORTIONMENT ; CHEMICAL SPECIATION ; EMISSION SOURCES ; INLAND SITES ; URBAN |
WOS研究方向 | Environmental Sciences & Ecology |
WOS类目 | Environmental Sciences |
语种 | 英语 |
出版者 | ELSEVIER SCI LTD |
WOS记录号 | WOS:000385596000029 |
内容类型 | 期刊论文 |
URI标识 | http://www.corc.org.cn/handle/1471x/2374778 |
专题 | 中国科学院大学 |
通讯作者 | Chen, Jinsheng |
作者单位 | 1.Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Urban Atmospher Environm, Xiamen 361021, Peoples R China 2.Chinese Acad Sci, Inst Urban Environm, Key Lab Urban Environm & Hlth, Xiamen 361021, Peoples R China 3.Chinese Acad Sci, NUEORS, Ningbo 315800, Zhejiang, Peoples R China 4.State Environm Protect Key Lab Cause & Prevent Ur, Shanghai 200233, Peoples R China 5.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Hong, Youwei,Chen, Jinsheng,Deng, Junjun,et al. Pattern of atmospheric mercury speciation during episodes of elevated pm2.5 levels in a coastal city in the yangtze river delta, china[J]. Environmental pollution,2016,218:259-268. |
APA | Hong, Youwei.,Chen, Jinsheng.,Deng, Junjun.,Tong, Lei.,Xu, Lingling.,...&Hong, Zhenyu.(2016).Pattern of atmospheric mercury speciation during episodes of elevated pm2.5 levels in a coastal city in the yangtze river delta, china.Environmental pollution,218,259-268. |
MLA | Hong, Youwei,et al."Pattern of atmospheric mercury speciation during episodes of elevated pm2.5 levels in a coastal city in the yangtze river delta, china".Environmental pollution 218(2016):259-268. |
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