Controllable deposition of TiO2nanopillars at room temperature for high performance perovskite solar cells with suppressed hysteresis
Huang, Aibin1,2; Lei, Lei1; Zhu, Jingting1,2; Yu, Yu1,2; Liu, Yan1; Yang, Songwang3; Bao, Shanhu1; Jin, Ping1,4
刊名Solar Energy Materials and Solar Cells
2017
卷号168页码:172-182
ISSN号09270248
DOI10.1016/j.solmat.2017.04.035
英文摘要A room temperature stratagy was proposed and realized for the fabrication of TiO2scaffold for perovskite solar cells (PSCs). By sueccetively sputtering TiO2, thermal evaporating PTFE template and sputtering TiO2again, bilayer TiO2electron extraction layer was prepared with controllable porosity. Owning to the high sputtering power, the electron transport layer consisting of compact layer and TiO2nanopillars was fully crystallized and no post thermal treatment was needed for the removal of PTFE template. The hysteresis of PSC was modulated and the porosity dependence of hysteresis was analyzed. PSC with a PCE of 15.08% and neglectable hysteresis was fabricated when the porosity of mesoporous scaffold was 45.77%. Our methodology offered a low cost room temperature scheme for the fabrication of mesostructured PSC. This approach makes large scale flexible PCS devices possible. What is more, this technique is versatile for the preparation of functional mesoporous materials with different pore structure and porosity requirements. © 2017
内容类型期刊论文
源URL[http://ir.sic.ac.cn/handle/331005/25826]  
专题中国科学院上海硅酸盐研究所
作者单位1.State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai institute of Ceramics, Chinese Academy of Sciences, Dingxi 1295, Changning, Shanghai; 200050, China;
2.University of Chinese Academy of Sciences, Yuquan 19, Shijingshan, Beijing; 100049, China;
3.CAS Key Laboratory of Materials for Energy Conversion, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Heshuo 588, Jiading, Shanghai; 201899, China;
4.National Institute of Advanced Industrial Science and Technology, Moriyama, Nagoya; 463-8560, Japan
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GB/T 7714
Huang, Aibin,Lei, Lei,Zhu, Jingting,et al. Controllable deposition of TiO2nanopillars at room temperature for high performance perovskite solar cells with suppressed hysteresis[J]. Solar Energy Materials and Solar Cells,2017,168:172-182.
APA Huang, Aibin.,Lei, Lei.,Zhu, Jingting.,Yu, Yu.,Liu, Yan.,...&Jin, Ping.(2017).Controllable deposition of TiO2nanopillars at room temperature for high performance perovskite solar cells with suppressed hysteresis.Solar Energy Materials and Solar Cells,168,172-182.
MLA Huang, Aibin,et al."Controllable deposition of TiO2nanopillars at room temperature for high performance perovskite solar cells with suppressed hysteresis".Solar Energy Materials and Solar Cells 168(2017):172-182.
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