A possible pathway for rapid growth of sulfate during haze days in China

doi:10.5194/acp-17-3301-2017

CORC > 地球环境研究所 > 中国科学院地球环境研究所 > 粉尘与环境研究室

	A possible pathway for rapid growth of sulfate during haze days in China
	Zhang, Qiang 1; Li, Guohui 4; Bei, Naifang 5; Cao, Junji 4; Huang, Rujin 4; Wu, Jiarui 4; Feng, Tian 4,5; Wang, Yichen 4; Liu, Suixin 4; Tie, Xuexi 4
刊名	ATMOSPHERIC CHEMISTRY AND PHYSICS
	2017-03-07
卷号	17 期号:5 页码:3301-3316
DOI	10.5194/acp-17-3301-2017
文献子类	Article
英文摘要	Rapid industrialization and urbanization have caused frequent occurrence of haze in China during wintertime in recent years. The sulfate aerosol is one of the most important components of fine particles (PM2.5) in the atmosphere, contributing significantly to the haze formation. However, the heterogeneous formation mechanism of sulfate remains poorly characterized. The relationships of the observed sulfate with PM2.5, iron, and relative humidity in Xi'an, China have been employed to evaluate the mechanism and to develop a parameterization of the sulfate heterogeneous formation involving aerosol water for incorporation into atmospheric chemical transport models. Model simulations with the proposed parameterization can successfully reproduce the observed sulfate rapid growth and diurnal variations in Xi'an and Beijing, China. Reasonable representation of sulfate heterogeneous formation in chemical transport models considerably improves the PM2.5 simulations, providing the underlying basis for better understanding the haze formation and supporting the design and implementation of emission control strategies.
WOS关键词	MEXICO-CITY ; MCMA-2006/MILAGRO CAMPAIGN ; HETEROGENEOUS REACTIONS ; PARTICULATE MATTER ; INORGANIC AEROSOLS ; ACID DEPOSITION ; URBAN FOG ; MODEL ; SO2 ; PHOTOCHEMISTRY
WOS研究方向	Meteorology & Atmospheric Sciences
语种	英语
WOS记录号	WOS:000396128600003
内容类型	期刊论文
源URL	[http://ir.ieecas.cn/handle/361006/5496]
专题	地球环境研究所_粉尘与环境研究室
作者单位	1.Tsinghua Univ, Dept Earth Syst Sci, Beijing, Peoples R China 2.MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA 3.Molina Ctr Energy & Environm, La Jolla, CA USA 4.Chinese Acad Sci, Inst Earth Environm, SKLLQG, Key Lab Aerosol Chem & Phys, Xian, Peoples R China 5.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian, Shaanxi, Peoples R China
推荐引用方式 GB/T 7714	Zhang, Qiang,Li, Guohui,Bei, Naifang,et al. A possible pathway for rapid growth of sulfate during haze days in China[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2017,17(5):3301-3316.
APA	Zhang, Qiang.,Li, Guohui.,Bei, Naifang.,Cao, Junji.,Huang, Rujin.,...&Molina, Luisa T..(2017).A possible pathway for rapid growth of sulfate during haze days in China.ATMOSPHERIC CHEMISTRY AND PHYSICS,17(5),3301-3316.
MLA	Zhang, Qiang,et al."A possible pathway for rapid growth of sulfate during haze days in China".ATMOSPHERIC CHEMISTRY AND PHYSICS 17.5(2017):3301-3316.