Widespread air pollutants of the North China Plain during the Asian summer monsoon season: a case study

doi:10.5194/acp-18-8491-2018

CORC > 地球环境研究所 > 中国科学院地球环境研究所 > 粉尘与环境研究室

	Widespread air pollutants of the North China Plain during the Asian summer monsoon season: a case study
	Tie, Xuexi 3; Wang, Yichen 3; Li, Guohui 3; Cao, Junji 3; Li, Xia 1,3; Bei, Naifang 2; Wu, Jiarui 1,3; Feng, Tian 3
刊名	ATMOSPHERIC CHEMISTRY AND PHYSICS
	2018-06-18
卷号	18 期号:12 页码:8491-8504
DOI	10.5194/acp-18-8491-2018
文献子类	Article
英文摘要	During the Asian summer monsoon season, prevailing southeasterly-southwesterly winds are subject to delivering air pollutants from the North China Plain (NCP) to northeast and northwest China. In the present study, the WRF-CHEM model is used to evaluate contributions of trans-boundary transport of NCP emissions to the air quality in northeast and northwest China during a persistent air pollution episode from 22 to 28 May 2015. The WRF-CHEM model generally performs well in capturing the observed temporal variation and spatial distribution of fine particulate matter (PM2.5), ozone (O-3), and NO2. The simulated temporal variation of aerosol species is also in good agreement with measurements in Beijing during the episode. Model simulations show that NCP emissions contribute substantially to the PM2.5 level in Liaoning and Shanxi provinces, the adjacent downwind areas of the NCP, with an average of 24.2 and 13.9 mu g m(-3) during the episode, respectively. The PM2.5 contributions in Jilin and Shanxi provinces are also appreciable, with an average of 9.6 and 6.5 mu g m(-3), respectively. The average percentage contributions of NCP emissions to the PM2.5 level in Liaoning, Jilin, Shanxi, and Shaanxi provinces are 40.6, 27.5, 32.2, and 20.9 %, respectively. The NCP emissions contribute remarkably to the O-3 level in Liaoning province, with an average of 46.5 mu g m(-3), varying from 23.9 to 69.5 mu g m(-3). The O-3 level in Shanxi province is also influenced considerably by NCP emissions, with an average contribution of 35.1 mu g m(-3). The O-3 level in Shanxi province is also influenced considerably by NCP emissions, with an average contribution of 35.1 mu g m(-3). The average O-3 contributions of NCP emissions to Jilin and Shaanxi provinces are 28.7 and 20.7 mu g m(-3), respectively. The average percentage contributions of NCP emissions to the afternoon O-3 level in Liaoning, Jilin, Shanxi, and Shaanxi provinces are 27.4, 19.5, 21.2, and 15.8 %, respectively. However, the effect of NCP emissions on the air quality in Inner Mongolia is generally insignificant. Therefore, effective mitigation of NCP emissions not only improves the local air quality, but is also beneficial to the air quality in northeast and northwest China during the Asian summer monsoon season.
WOS关键词	CAL-MEX 2010 ; METEOROLOGICAL UNCERTAINTIES ; MCMA-2006/MILAGRO CAMPAIGN ; AEROSOL CONCENTRATIONS ; SOURCE APPORTIONMENT ; FACTOR SEPARATION ; OZONE FORMATION ; FIELD CAMPAIGN ; HAZE FORMATION ; EASTERN CHINA
WOS研究方向	Meteorology & Atmospheric Sciences
语种	英语
WOS记录号	WOS:000435484300002
内容类型	期刊论文
源URL	[http://ir.ieecas.cn/handle/361006/5094]
专题	地球环境研究所_粉尘与环境研究室
通讯作者	Li, Guohui
作者单位	1.Univ Chinese Acad Sci, Beijing, Peoples R China 2.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian, Shaanxi, Peoples R China 3.Chinese Acad Sci, Key Lab Aerosol Chem & Phys, SKLLQG, Inst Earth Environm, Xian, Shaanxi, Peoples R China
推荐引用方式 GB/T 7714	Tie, Xuexi,Wang, Yichen,Li, Guohui,et al. Widespread air pollutants of the North China Plain during the Asian summer monsoon season: a case study[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(12):8491-8504.
APA	Tie, Xuexi.,Wang, Yichen.,Li, Guohui.,Cao, Junji.,Li, Xia.,...&Feng, Tian.(2018).Widespread air pollutants of the North China Plain during the Asian summer monsoon season: a case study.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(12),8491-8504.
MLA	Tie, Xuexi,et al."Widespread air pollutants of the North China Plain during the Asian summer monsoon season: a case study".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.12(2018):8491-8504.