The Potential of Cu-SAPO-44 in the Selective Catalytic Reduction of NOxwith NH3

doi:10.1002/cctc.201601159

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	The Potential of Cu-SAPO-44 in the Selective Catalytic Reduction of NOxwith NH3
	Xin, Ying 1; Wang, Xiao 1; Li, Qian 1; Ma, Xicheng 2; Qi, Yongxin 3; Zheng, Lirong4 ; Anderson, James A.5; Zhang, Zhaoliang 1; Zhang XD(张旭东); Liu Y(刘元)
刊名	ChemCatChem
	2016
卷号	8 期号:24 页码:3740-3745-
DOI	10.1002/cctc.201601159
文献子类	期刊论文
英文摘要	Nitrogen oxides (NOx) contribute much to acid rain, photochemical smog, and the depletion of tropospheric ozone. A novel, small-pore Cu-exchanged chabazite (Cu-CHA) zeolite, Cu-SAPO-44, was first studied for the selective catalytic reduction of NOxwith ammonia (NH3-SCR), and exhibits excellent activity and N2selectivity over the wide temperature window from 200鈥?50 掳C. The Cu content in Cu-SAPO-44 plays a significant role in the NH3-SCR reactions. Two kinds of isolated Cu2+species inside the large cages and in the six-membered rings of the CHA structure were verified as the active sites, which are responsible for the low-temperature and high-temperature activity, respectively. Cu-SAPO-44 is shown to be a promising candidate as a SCR catalyst for deNOxwith great potential in after-treatment systems for either mobile or stationary sources. 漏 2016 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim
语种	英语
内容类型	期刊论文
源URL	[http://ir.ihep.ac.cn/handle/311005/260355]
专题	高能物理研究所_粒子天体物理中心高能物理研究所_多学科研究中心
作者单位	1.济南大学化学化工学院氟化学与特种化工材料实验室 2.山东大学化学与化工学院 3.School of Material Science and Technology, Shandong University, Jinan 4.中国科学院高能物理研究所 5.Materials and Chemical Engineering Group, School of Engineering, University of Aberdeen, Aberdeen 6.AB24 3UE, United Kingdom
推荐引用方式 GB/T 7714	Xin, Ying,Wang, Xiao,Li, Qian,et al. The Potential of Cu-SAPO-44 in the Selective Catalytic Reduction of NOxwith NH3[J]. ChemCatChem,2016,8(24):3740-3745-.
APA	Xin, Ying.,Wang, Xiao.,Li, Qian.,Ma, Xicheng.,Qi, Yongxin.,...&刘元.(2016).The Potential of Cu-SAPO-44 in the Selective Catalytic Reduction of NOxwith NH3.ChemCatChem,8(24),3740-3745-.
MLA	Xin, Ying,et al."The Potential of Cu-SAPO-44 in the Selective Catalytic Reduction of NOxwith NH3".ChemCatChem 8.24(2016):3740-3745-.