On the source contribution to Beijing PM2.5 concentrations
Zikova, Nadezda1; Wang, Yungang2; Yang, Fumo3; Li, Xinghua4; Tian, Mi3; Hopke, Philip K.1
刊名ATMOSPHERIC ENVIRONMENT
2016-06-01
卷号134页码:84-95
关键词Beijing Positive Matrix Factorization Pm2.5 Traffic Coal Combustion
ISSN号1352-2310
DOI10.1016/j.atmosenv.2016.03.047
英文摘要

Beijing is a city with some of the world's worst particulate air pollution. Although there have been various control strategies implemented since 1998, there are still episodes of PM2.5 concentrations of hundreds of micrograms per cubic meter. In this study, samples were collected over a year in Beijing, chemically characterized, and the resulting data analyzed for source apportionment. The new error analysis capabilities built into EPA PMF V5.0 have been employed to better evaluate the profiles and assign them to source types. Secondary sulfate, local coal combustion and secondary nitrate were the major contributors to the PM2.5 mass. However, in this study, traffic was found to be more important as a PM compared to prior studies. It was actually the largest PM2.5 source in autumn and winter although local coal combustion is also a large source of PM in the winter months. These results demonstrate the value of using the displacement method to assess the variability in source profiles to improve our interpretation of PMF results. They also suggest more attention needs to be paid to traffic emissions in Beijing. (C) 2016 Elsevier Ltd. All rights reserved.

资助项目National Natural Science Foundation of China projects[41275121] ; National Natural Science Foundation of China projects[41575119] ; National Natural Science Foundation of China projects[41075093] ; National Natural Science Foundation of China projects[41375123]
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
语种英语
出版者PERGAMON-ELSEVIER SCIENCE LTD
WOS记录号WOS:000375504100009
内容类型期刊论文
源URL[http://119.78.100.138/handle/2HOD01W0/2444]  
专题大气环境研究中心
作者单位1.Clarkson Univ, Potsdam, NY 13699 USA
2.GAGO Inc, San Jose, CA USA
3.Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China
4.Beihang Univ, Sch Space & Environm, Beijing 100191, Peoples R China
推荐引用方式
GB/T 7714
Zikova, Nadezda,Wang, Yungang,Yang, Fumo,et al. On the source contribution to Beijing PM2.5 concentrations[J]. ATMOSPHERIC ENVIRONMENT,2016,134:84-95.
APA Zikova, Nadezda,Wang, Yungang,Yang, Fumo,Li, Xinghua,Tian, Mi,&Hopke, Philip K..(2016).On the source contribution to Beijing PM2.5 concentrations.ATMOSPHERIC ENVIRONMENT,134,84-95.
MLA Zikova, Nadezda,et al."On the source contribution to Beijing PM2.5 concentrations".ATMOSPHERIC ENVIRONMENT 134(2016):84-95.
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