A New kHz Velocity Map Ion/Electron Imaging Spectrometer for Femtosecond Time-Resolved Molecular Reaction Dynamics Studies | |
He, Zhi-gang1,2; Chen, Zhi-chao1,2; Yan, Dong-yuan1,2; Dai, Dong-xu1; Wu, Guo-rong1; Yang, Xue-ming1 | |
刊名 | CHINESE JOURNAL OF CHEMICAL PHYSICS
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2017-06-01 | |
卷号 | 30期号:3页码:247-252 |
关键词 | Photoelectron Spectrum Pump/probe Femtosecond Time-resolved |
DOI | 10.1063/1674-0068/30/cjcp1702018 |
英文摘要 | A new velocity map imaging spectrometer is constructed for molecular reaction dynamics studies using time-resolved photoelectron/ion spectroscopy method. By combining a kHz pulsed valve and an ICCD camera, this velocity map imaging spectrometer can be run at a repetition rate of 1 kHz, totally compatible with the fs Ti:Sapphire laser system, facilitating time-resolved studies in gas phase which are usually time-consuming. Time-resolved velocity map imaging study of NH3 photodissociation at 200 nm was performed and the time-resolved total kinetic energy release spectrum of H+NH2 products provides rich information about the dissociation dynamics of NH3. These results show that this new apparatus is a powerful tool for investigating the molecular reaction dynamics using time-resolved methods. |
语种 | 英语 |
WOS记录号 | WOS:000405446400002 |
内容类型 | 期刊论文 |
源URL | [http://cas-ir.dicp.ac.cn/handle/321008/152028] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
作者单位 | 1.Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | He, Zhi-gang,Chen, Zhi-chao,Yan, Dong-yuan,et al. A New kHz Velocity Map Ion/Electron Imaging Spectrometer for Femtosecond Time-Resolved Molecular Reaction Dynamics Studies[J]. CHINESE JOURNAL OF CHEMICAL PHYSICS,2017,30(3):247-252. |
APA | He, Zhi-gang,Chen, Zhi-chao,Yan, Dong-yuan,Dai, Dong-xu,Wu, Guo-rong,&Yang, Xue-ming.(2017).A New kHz Velocity Map Ion/Electron Imaging Spectrometer for Femtosecond Time-Resolved Molecular Reaction Dynamics Studies.CHINESE JOURNAL OF CHEMICAL PHYSICS,30(3),247-252. |
MLA | He, Zhi-gang,et al."A New kHz Velocity Map Ion/Electron Imaging Spectrometer for Femtosecond Time-Resolved Molecular Reaction Dynamics Studies".CHINESE JOURNAL OF CHEMICAL PHYSICS 30.3(2017):247-252. |
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