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	Performance and mechanism of hierarchically porous Ce-Zr oxide nanospheres encapsulated calcium alginate beads for fluoride removal from water
	Chen, Liang1,2; Zhang, Kaisheng1,2; He, Junyong1,2; Cai, Xing-Guo1,2; Xu, Weihong1,2; Liu, Jin-Huai1,2
刊名	RSC ADVANCES
	2016
卷号	6期号:43页码:36296-36306
DOI	10.1039/c6ra01337f
文献子类	Article
英文摘要	Hierarchically porous Ce-Zr oxide nanosphere encapsulated calcium alginate millimeter-sized beads (CZ-CABs) were synthesized by using a sol-gel templating technique. Their defluoridation performance, including static and dynamic adsorption, was systematically evaluated. The adsorption kinetic followed the pseudo-second-order model. The adsorption isotherm could be divided into two distinct regions depending on the fluoride concentrations, and the CZ-CABs exhibited a Langmuir-Freundlich maximum fluoride adsorption capacity of 137.6 mg g(-1) under neutral conditions. Such a specific adsorption isotherm indicated that various mechanisms were involved in the fluoride adsorption depending on fluoride concentrations, which were further demonstrated by FTIR and XPS analyses. The effect of pH and co-existing anions on fluoride adsorption was studied. Furthermore, column adsorption experiments were conducted, and the results showed a high efficiency of the CZ-CABs for the removal of fluoride from water on a continuous flow basis.
WOS关键词	DRINKING-WATER ; AQUEOUS-SOLUTION ; ADSORPTION MECHANISM ; CHITOSAN BEADS ; PHOTOCATALYTIC ACTIVITY ; IMPREGNATED CHITOSAN ; ACTIVATED CARBON ; ARSENIC REMOVAL ; TIO2 POWDERS ; ADSORBENT
WOS研究方向	Chemistry
语种	英语
WOS记录号	WOS:000374561300012
资助机构	National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; Natural Science Foundation of China(21277146 ; Natural Science Foundation of China(21277146 ; Natural Science Foundation of China(21277146 ; Natural Science Foundation of China(21277146 ; Anhui Major Technological Program(1501021005) ; Anhui Major Technological Program(1501021005) ; Anhui Major Technological Program(1501021005) ; Anhui Major Technological Program(1501021005) ; U1432131) ; U1432131) ; U1432131) ; U1432131) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; Natural Science Foundation of China(21277146 ; Natural Science Foundation of China(21277146 ; Natural Science Foundation of China(21277146 ; Natural Science Foundation of China(21277146 ; Anhui Major Technological Program(1501021005) ; Anhui Major Technological Program(1501021005) ; Anhui Major Technological Program(1501021005) ; Anhui Major Technological Program(1501021005) ; U1432131) ; U1432131) ; U1432131) ; U1432131)
内容类型	期刊论文
源URL	[http://ir.hfcas.ac.cn:8080/handle/334002/22397]
专题	合肥物质科学研究院_中科院合肥智能机械研究所
作者单位	1.Chinese Acad Sci, Inst Intelligent Machines, Nanomat & Environm Detect Lab, Hefei 230031, Anhui, Peoples R China 2.Univ Sci & Technol China, Dept Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China
推荐引用方式 GB/T 7714	Chen, Liang,Zhang, Kaisheng,He, Junyong,et al. Performance and mechanism of hierarchically porous Ce-Zr oxide nanospheres encapsulated calcium alginate beads for fluoride removal from water[J]. RSC ADVANCES,2016,6(43):36296-36306.
APA	Chen, Liang,Zhang, Kaisheng,He, Junyong,Cai, Xing-Guo,Xu, Weihong,&Liu, Jin-Huai.(2016).Performance and mechanism of hierarchically porous Ce-Zr oxide nanospheres encapsulated calcium alginate beads for fluoride removal from water.RSC ADVANCES,6(43),36296-36306.
MLA	Chen, Liang,et al."Performance and mechanism of hierarchically porous Ce-Zr oxide nanospheres encapsulated calcium alginate beads for fluoride removal from water".RSC ADVANCES 6.43(2016):36296-36306.

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