Raspberry-like Hierarchical Au/Pt Nanoparticle Assembling Hollow Spheres with Nanochannels: An Advanced Nanoelectrocatalyst for the Oxygen Reduction Reaction | |
Guo SJ ; Dong SJ ; Wang EK | |
刊名 | journal of physical chemistry c
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2009 | |
卷号 | 113期号:14页码:5485-5492 |
关键词 | HYBRID NANOSTRUCTURES ENHANCED CATALYSIS CONTROLLED-RELEASE FACILE SYNTHESIS SILICA SPHERES PLATINUM NANOCRYSTALS NANORODS ELECTROCATALYST MONODISPERSE |
ISSN号 | 1932-7447 |
通讯作者 | wang ek |
中文摘要 | in this contribution, we for the first time report the synthesis of raspberry-like hierarchical au/pt nanoparticle (np) assembling hollow spheres (rhahs) with pore structure and complex morphology through one in situ sacrificial template approach without any post-treatment procedure. this method has some clear advantages including simplicity, quickness, high quality, good reproducibility, and no need of a complex post-treatment process (removing templating). furthermore, the present method could be extended to other metal-based np assembling hollow spheres. most importantly, the as-prepared rhahs exhibited excellent electrocatalytic activity for oxygen reduction reaction (orr). for instance, the present rhahs-modified electrode exhibited more positive potential (the half-wave potential at about 0.6 v), higher specific activity, and higher mass activity for orr than that of commercial platinum black (cpb). rotating ring-disk electrode (rrde) voltarnmetry demonstrated that the rhahs-modified electrode could almost catalyze a four-electron reduction of o-2 to h2o in a 0.5 m air-saturated h2so4 solution. |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000264805700024 |
公开日期 | 2010-06-18 |
内容类型 | 期刊论文 |
源URL | [http://202.98.16.49/handle/322003/12693] ![]() |
专题 | 长春应用化学研究所_长春应用化学研究所知识产出_期刊论文 |
推荐引用方式 GB/T 7714 | Guo SJ,Dong SJ,Wang EK. Raspberry-like Hierarchical Au/Pt Nanoparticle Assembling Hollow Spheres with Nanochannels: An Advanced Nanoelectrocatalyst for the Oxygen Reduction Reaction[J]. journal of physical chemistry c,2009,113(14):5485-5492. |
APA | Guo SJ,Dong SJ,&Wang EK.(2009).Raspberry-like Hierarchical Au/Pt Nanoparticle Assembling Hollow Spheres with Nanochannels: An Advanced Nanoelectrocatalyst for the Oxygen Reduction Reaction.journal of physical chemistry c,113(14),5485-5492. |
MLA | Guo SJ,et al."Raspberry-like Hierarchical Au/Pt Nanoparticle Assembling Hollow Spheres with Nanochannels: An Advanced Nanoelectrocatalyst for the Oxygen Reduction Reaction".journal of physical chemistry c 113.14(2009):5485-5492. |
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