包覆型非贵金属氧还原催化剂的研究进展

CORC > 厦门大学 > 2016年第22卷

	包覆型非贵金属氧还原催化剂的研究进展; Recent Progress in Non-Precious Metal Oxygen Reduction Reaction Catalysts with an Encapsulation Structure
	肖梅玲 ; 祝建兵 ; 刘长鹏 ; 葛君杰 ; 邢巍 ; XIAO Mei-ling ; ZHU Jian-bing ; LIU Chang-peng ; GE Jun-jie ; XING Wei
刊名	http://electrochem.xmu.edu.cn/CN/abstract/abstract10261.shtml
	2016-05-03
关键词	氧还原反应过渡金属包覆非贵金属催化剂 oxygen reduction reaction transition-metals encased non-precious metal catalysts
英文摘要	燃料电池中广泛使用的铂基催化剂价格昂贵、储量低、容易失活，因此亟待开发廉价、高效非铂催化剂. 过渡金属(Fe、Co、Ni等)/杂原子共掺杂催化剂、杂原子掺杂（N、P、S、F等）碳材料以及碳材料包覆过渡金属复合物是目前发现的几类性能优异的非贵金属氧还原催化剂. 其中碳材料包覆过渡金属催化剂作为一类新型的高性能催化剂，对其研究还有待深入. 本文主要阐述了国内外在包覆型非贵金属氧还原催化剂方面的研究进展，从合成，性能，机理等方面对该类催化剂进行了总结，力求助益于该类催化剂的发展.; Platinum-based materials, the state-of-the-art catalysts for fuel cells, suffer from prohibitive costs, limited resources and insufficient durability. Accordingly, tremendous efforts were made in searching for efficient, durable and inexpensive alternatives to precious-metal electrocatalysts for the oxygen reduction reaction (ORR). Transition-metals (Fe, Co)/nitrogen co-doped hybrids, heteroatom (N, P, S, F, et al) doped carbons and composites with transition-metals encapsulated in graphitic layers are reported as the most efficient non-precious metal ORR catalysts. Among the various non-precious metal ORR catalysts, transition-metals encased in graphitic layer catalysts are a novel type of catalysts for ORR with high activity and durability, and thus, the in-depth researches are highly desirable. Here, we present the recent research progress in transition-metals encased catalysts from the aspects of synthesis, activity and catalytic mechanism, in an effort to promote the developments of these catalysts.; 科技部973项目（No. 2012CB215500）、国家自然科学基金项目（No. 21373199，No. 21433003）、中国科学院先导专项（No. XDA09030104）、吉林省科技发展项目（No. 20130206068GX，No. 20140203012SF，No. 20102204）和吉林省自然科学基金项目（No. 20150101066JC）资助; 作者联系地址：1. 中国科学院长春应用化学研究所，电分析国家重点实验室，吉林长春 130022；2. 中国科学院长春应用化学研究所，先进化学电源实验室，吉林长春 130022; Author's Address: 1. State Key Laboratory of Electroanalytical Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China; 2. Laboratory of Advanced Power Sources, Changchun Institute of Applied Chemistry, Changchun 130022, China; 通讯作者E-mail：xingwei@ciac.ac.cn
语种	中文
出版者	厦门大学《电化学》编辑部
内容类型	期刊论文
源URL	[http://dx.doi.org/10.13208/j.electrochem.151152]
专题	2016年第22卷
推荐引用方式 GB/T 7714	肖梅玲,祝建兵,刘长鹏,等. 包覆型非贵金属氧还原催化剂的研究进展, Recent Progress in Non-Precious Metal Oxygen Reduction Reaction Catalysts with an Encapsulation Structure[J]. http://electrochem.xmu.edu.cn/CN/abstract/abstract10261.shtml,2016.
APA	肖梅玲.,祝建兵.,刘长鹏.,葛君杰.,邢巍.,...&XING Wei.(2016).包覆型非贵金属氧还原催化剂的研究进展.http://electrochem.xmu.edu.cn/CN/abstract/abstract10261.shtml.
MLA	肖梅玲,et al."包覆型非贵金属氧还原催化剂的研究进展".http://electrochem.xmu.edu.cn/CN/abstract/abstract10261.shtml (2016).