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Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression
Iwamoto, M. ; Wu, C. X. ; Zhong-Can, O. Y. ; Wu CX(吴晨旭)
2000
关键词CIRCULAR-DICHROISM SPECTROSCOPY OPTICAL 2ND-HARMONIC GENERATION 2ND HARMONIC-GENERATION MOLECULAR-ORIENTATION ROTATIONAL AVERAGES SURFACE FILMS
英文摘要The complete expression for the macroscopic second-order susceptibility (SOS) tensor chi((2)) for a monolayer with C-infinity symmetry at the air-liquid interface is derived as functions of the molecular SOS tensor alpha((2)) and the orientational order parameters. The chiral (non-chiral) terms of chi((2)) distinguished by their association with even (odd) order parameters, by which a second-harmonic generation (SHG) circular-dichroism effect can be better understood. An SHG experiment of a 4-cyano-4'-5-alkyl-biphenyl monolayer on an air-water interface by monolayer compression is also discussed. (C) 2000 Elsevier Science B.V. All rights reserved.
语种英语
内容类型期刊论文
源URL[http://dspace.xmu.edu.cn/handle/2288/68813]  
专题物理技术-已发表论文
推荐引用方式
GB/T 7714
Iwamoto, M.,Wu, C. X.,Zhong-Can, O. Y.,et al. Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression[J],2000.
APA Iwamoto, M.,Wu, C. X.,Zhong-Can, O. Y.,&吴晨旭.(2000).Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression..
MLA Iwamoto, M.,et al."Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression".(2000).
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