Band edge emission enhancement by quadrupole surface plasmon-exciton coupling using direct-contact Ag/ZnO nanospheres

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	Band edge emission enhancement by quadrupole surface plasmon-exciton coupling using direct-contact Ag/ZnO nanospheres
	Zang, Yashu ; He, Xu ; Li, Jing ; Yin, Jun ; Li, Kongyi ; Yue, Chuang ; Wu, Zhiming ; Wu, Suntao ; Kang, Junyong ; Wu ZM(吴志明)
刊名	http://dx.doi.org/10.1039/c2nr32906a
	2013
关键词	SILVER SURFACE QUANTUM-WELLS SOLAR-CELLS NANOPARTICLES ARRAYS PHOTOLUMINESCENCE SPECTROSCOPY SIZE
英文摘要	Periodic Ag nanoball (NB) arrays on ZnO hollow nanosphere (HNS) supporting structures were fabricated in a large area by a laser irradiation method. The optimized laser power and spherical supporting structure of ZnO with a certain size and separation were employed to aggregate a sputtering-deposited Ag nano-film into an ordered, large-area, and two dimensional Ag NB array. A significant band edge (BE) emission enhancement of ZnO HNSs was achieved on this Ag NB/ZnO HNS hybrid structure and the mechanism was revealed by further experimental and theoretical analyses. With successfully fabricating the direct-contact structure of a Ag NB on the top of each ZnO HNS, the highly localized quadrupole mode surface plasmon resonance (SPR), realized on the metal NBs in the ultraviolet region, can effectively improve the BE emission of ZnO through strong coupling with the excitons of ZnO. Compared with the dipole mode SPR, the quadrupole mode SPR is insensitive to the metal nanoparticle's size and has a resonance frequency in the BE region of the wide band gap materials, hence, it can be potentially applied in related optoelectronic devices.
语种	英语
内容类型	期刊论文
源URL	[http://dspace.xmu.edu.cn/handle/2288/68743]
专题	物理技术－已发表论文
推荐引用方式 GB/T 7714	Zang, Yashu,He, Xu,Li, Jing,et al. Band edge emission enhancement by quadrupole surface plasmon-exciton coupling using direct-contact Ag/ZnO nanospheres[J]. http://dx.doi.org/10.1039/c2nr32906a,2013.
APA	Zang, Yashu.,He, Xu.,Li, Jing.,Yin, Jun.,Li, Kongyi.,...&吴志明.(2013).Band edge emission enhancement by quadrupole surface plasmon-exciton coupling using direct-contact Ag/ZnO nanospheres.http://dx.doi.org/10.1039/c2nr32906a.
MLA	Zang, Yashu,et al."Band edge emission enhancement by quadrupole surface plasmon-exciton coupling using direct-contact Ag/ZnO nanospheres".http://dx.doi.org/10.1039/c2nr32906a (2013).