Complete oxidation of methane on Co3O4-SnO2 catalysts | |
Tang, Xingfu ; Hao, Jiming ; Li, Junhua | |
2010-10-12 ; 2010-10-12 | |
关键词 | Co3O4-SnO2 complete oxidation methane (CH4) LOW-TEMPERATURE SENSING PROPERTIES ROOM-TEMPERATURE SUPPORTED COBALT COMBUSTION COMPOSITES REDUCTION SENSOR ZRO2 CO Engineering, Environmental Environmental Sciences |
中文摘要 | Co3O4-SnO2 hybrid oxides were prepared by the coprecipitation method and were used to oxidate methane (CH4) in presence of oxygen. The Co3O4-SnO2 with a molar ratio of Co/(Co + Sn) at 0.75 exhibited the highest catalytic activity among all the Co3O4-SnO2 hybrid oxides. Experimental results showed that the catalysts were considerably stable in the CH4 combustion reaction, and were verified by X-ray photoelectron spectra (XPS). It was found that Co3O4 was the active species, and SnO2 acted as a support or a promoting component in the Co3O4-SnO2 hybrid oxides. The surface area was not a major factor that affected catalytic activity. The hydrogen temperature-programmed reduction (H-2-TPR) results demonstrated that the interaction between cobalt and tin oxides accelerated the mobility of oxygen species of Co3O4-SnO2, leading to higher catalytic activity. |
语种 | 英语 ; 英语 |
出版者 | HIGHER EDUCATION PRESS ; BEIJING ; SHATANHOU ST 55, BEIJING 100009, PEOPLES R CHINA |
内容类型 | 期刊论文 |
源URL | [http://hdl.handle.net/123456789/79669] ![]() |
专题 | 清华大学 |
推荐引用方式 GB/T 7714 | Tang, Xingfu,Hao, Jiming,Li, Junhua. Complete oxidation of methane on Co3O4-SnO2 catalysts[J],2010, 2010. |
APA | Tang, Xingfu,Hao, Jiming,&Li, Junhua.(2010).Complete oxidation of methane on Co3O4-SnO2 catalysts.. |
MLA | Tang, Xingfu,et al."Complete oxidation of methane on Co3O4-SnO2 catalysts".(2010). |
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