Effects of Metallic Heating Plates on Coal Pyrolysis Behavior in a Fixed-Bed Reactor Enhanced with Internals | |
Hu, Erfeng1,2,3; Zeng, Xi2; Wang, Fang2; Li, Yuan3; Yi, Xiaojian4; Fu, Xiaoheng1 | |
刊名 | ENERGY & FUELS |
2017-03-01 | |
卷号 | 31期号:3页码:2716-2721 |
ISSN号 | 0887-0624 |
DOI | 10.1021/acs.energyfuels.6b02975 |
文献子类 | Article |
英文摘要 | A newly configured fixed-bed reactor with internals has been proposed to enhance the coal pyrolysis performance. In this study, the effects of metallic plates on coal pyrolysis behavior were investigated in this reactor. The results show that the increased quantity of the metallic plates enhanced the heat transfer and shortened the residence time of volatiles within the coal particles. In addition, the pressure drop results suggest that the increased quantity of plates caused short circuiting of gas and raised the particle interstices, which reduced the gas diffusion resistance of pyrolysis products. Therefore, more gaseous pyrolysis products flowed into central low-temperature coal bed and escaped from the gas collection pipe, suppressing the secondary reaction of pyrolysis products and increasing the tar yield and quality. At a furnace temperature of 900 degrees C, the increase in metallic plates from 0 to 8 raised the tar yield and light tar fraction from 5.20 and 69.5 wt % to 7.86 and 77.0 wt %, respectively. Meanwhile, the <= C-14 hydrocarbons were elevated from 42.11 to 50.44 wt %, but the >= C-20 hydrocarbons were lowered from 29.95 to 19.74 wt %. However, an excessive increase in plates raised the heating rate of coal, cracking more pyrolysis products and decreasing the tar yield and quality. |
WOS关键词 | Oil-shale Pyrolysis ; High-quality Tar ; In-situ ; Gasification ; Conversion ; Oxidation ; Pressure ; Moisture ; Removal ; Chars |
WOS研究方向 | Energy & Fuels ; Engineering |
语种 | 英语 |
WOS记录号 | WOS:000396970400063 |
资助机构 | National High-Tech Research and Development Projects(2015AA050505-02) ; Major Program of the National Natural Science Foundation of China(U1302273) |
内容类型 | 期刊论文 |
源URL | [http://ir.ipe.ac.cn/handle/122111/22090] |
专题 | 过程工程研究所_多相复杂系统国家重点实验室 |
作者单位 | 1.China Univ Min & Technol Beijing, Sch Chem & Environm Engn, Beijing 100083, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 3.Univ New Brunswick, Dept Chem Engn, Fredericton, NB E3B 5A3, Canada 4.China North Ind Grp Corp, Res Inst 1, Dept Overall Technol, Beijing 100072, Peoples R China |
推荐引用方式 GB/T 7714 | Hu, Erfeng,Zeng, Xi,Wang, Fang,et al. Effects of Metallic Heating Plates on Coal Pyrolysis Behavior in a Fixed-Bed Reactor Enhanced with Internals[J]. ENERGY & FUELS,2017,31(3):2716-2721. |
APA | Hu, Erfeng,Zeng, Xi,Wang, Fang,Li, Yuan,Yi, Xiaojian,&Fu, Xiaoheng.(2017).Effects of Metallic Heating Plates on Coal Pyrolysis Behavior in a Fixed-Bed Reactor Enhanced with Internals.ENERGY & FUELS,31(3),2716-2721. |
MLA | Hu, Erfeng,et al."Effects of Metallic Heating Plates on Coal Pyrolysis Behavior in a Fixed-Bed Reactor Enhanced with Internals".ENERGY & FUELS 31.3(2017):2716-2721. |
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