Characterization of Polycyclic Aromatic Hydrocarbons in Cloud Deposition at Mount Heng in Southern China
Li, Peng-Hui; Wang, Yan; Li, Yu-Hua; Yang, Min-Min; Sun, Ming-Hu; Guo, Jia; Shou, You-Ping; Yi, Xianliang; Wang, Lei; Xi, Zhi-Lin
刊名AEROSOL AND AIR QUALITY RESEARCH
2016-12
卷号16期号:12页码:3164-3174
关键词Cloud water PAHs Scavenging ratio Transport pattern Source analysis
英文摘要Cloud water samples were collected during March to May 2009 at Mount Heng (27 degrees 18'N, 112 degrees 42'E, 1269 m A.S.L.), a high altitude site in southern China. The samples were analyzed by GS-MS to investigate the distribution, transport pattern, scavenging ratios and possible sources of PAHs. During the observation campaign, the concentration of total (in both particle and dissolved phase) PAHs in cloud water ranged from 323.0-5660 ng L-1, with an average of 1589 ng L-1. BbF was the most abundant compound, contributing to 14.50% of the total PAH concentration, followed by PhA, FluA, Pyr, BaA and Chr. Particle scavenging (Wp) was the dominate removal mechanism, accounting for over 77% of the total scavenging. Significant negative relationship was found between logWp and supercooled vapor pressure of PAHs, suggesting that particle scavenging by cloud water is more efficient for higher molecular weight PAHs. During the observation period, air mass was suggested to mainly originate from south or southeast of China based on back trajectory analysis, while air masses coming from northern China had highest PAH concentration. Diagnostic ratio and principal component analysis indicated that PAHs in cloud water at Mount Heng might originate from multiple sources.
收录类别SCI
内容类型期刊论文
源URL[http://ir.rcees.ac.cn/handle/311016/35816]  
专题生态环境研究中心_环境化学与生态毒理学国家重点实验室
推荐引用方式
GB/T 7714
Li, Peng-Hui,Wang, Yan,Li, Yu-Hua,et al. Characterization of Polycyclic Aromatic Hydrocarbons in Cloud Deposition at Mount Heng in Southern China[J]. AEROSOL AND AIR QUALITY RESEARCH,2016,16(12):3164-3174.
APA Li, Peng-Hui.,Wang, Yan.,Li, Yu-Hua.,Yang, Min-Min.,Sun, Ming-Hu.,...&Li, Zhi-Yong.(2016).Characterization of Polycyclic Aromatic Hydrocarbons in Cloud Deposition at Mount Heng in Southern China.AEROSOL AND AIR QUALITY RESEARCH,16(12),3164-3174.
MLA Li, Peng-Hui,et al."Characterization of Polycyclic Aromatic Hydrocarbons in Cloud Deposition at Mount Heng in Southern China".AEROSOL AND AIR QUALITY RESEARCH 16.12(2016):3164-3174.
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