Heterogeneous uptake of gaseous hydrogen peroxide on mineral dust | |
Zhou, Li; Wang, Weigang; Ge, Maofa; Tong, Shengrui | |
刊名 | JOURNAL OF ENVIRONMENTAL SCIENCES
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2016-02-01 | |
卷号 | 40页码:44-50 |
关键词 | Hydrogen peroxide Mineral dust Heterogeneous uptake Uptake coefficients |
英文摘要 | The heterogeneous uptake processes of hydrogen peroxide on Arizona test dust and two types of authentic Chinese mineral dusts, i.e., Inner Mongolia desert dust and Xinjiang calciferous dust, were investigated using a Knudsen cell reactor coupled with a quadrupole mass spectrometer. The uptake coefficients were measured as a function of the initial concentration of H2O2 from 2.6 x 10(11) to 1.2 x 10(12) molecules/cm(3), and the temperature dependence of the uptake coefficients was investigated over a range from 253 to 313 K. The concentration of H2O2 showed little effect on the uptake coefficients of these heterogeneous processes. As a function of temperature, the initial uptake coefficients decrease with increasing temperature, whereas the steady state uptake coefficients of Arizona test dust and Inner Mongolia desert dust increase with increasing temperature. Implications for the understanding of the uptake processes onto mineral dust samples were also discussed. (C) 2015 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V. |
收录类别 | SCI ; ISTP |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.iccas.ac.cn/handle/121111/36026] ![]() |
专题 | 化学研究所_分子动态与稳态结构实验室 |
作者单位 | Chinese Acad Sci, Inst Chem, State Key Lab Struct Chem Unstable & Stable Speci, BNLMS, Beijing 100190, Peoples R China |
推荐引用方式 GB/T 7714 | Zhou, Li,Wang, Weigang,Ge, Maofa,et al. Heterogeneous uptake of gaseous hydrogen peroxide on mineral dust[J]. JOURNAL OF ENVIRONMENTAL SCIENCES,2016,40:44-50. |
APA | Zhou, Li,Wang, Weigang,Ge, Maofa,&Tong, Shengrui.(2016).Heterogeneous uptake of gaseous hydrogen peroxide on mineral dust.JOURNAL OF ENVIRONMENTAL SCIENCES,40,44-50. |
MLA | Zhou, Li,et al."Heterogeneous uptake of gaseous hydrogen peroxide on mineral dust".JOURNAL OF ENVIRONMENTAL SCIENCES 40(2016):44-50. |
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