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	Influence of Exciton Localization on the Emission and Ultraviolet Photoresponse of ZnO/ZnS Core-Shell Nanowires
	Fang, X.; Z. P. Wei; R. Chen; J. L. Tang; H. F. Zhao; L. G. Zhang; D. X. Zhao; D. Fang; J. H. Li; F. Fang
刊名	Acs Applied Materials & Interfaces
	2015
卷号	7期号:19页码:10331-10336
英文摘要	The structural and optical properties of ZnO and ZnO/ ZnS core shell nanowires grown by a wet chemical method are investigated. The near-bandgap ultraviolet (UV) emission of the ZnO nanowires was enhanced by four times after coating with ZnS. The enhanced emission was attributed to surface passivation Of the ZnO nanowires and localized states introduced during ZnS growth. The emission of the ZnO and ZnO/ZnS core shell nanowires was attributed to neutral donor-bound excitons and localized excitons, respectively. Localized states prevented excitons from diffusing to nonradiative recombination centers, so therefore contributed to the enhanced emission. Emission from the localized exciton was not sensitive to temperature, so emission from the ZnO/ZnS core shell nanowires was more stable at higher temperature. UV photodetectors based on the ZnO and ZnO/ZnS core shell nanowires were fabricated. Under UV excitation, the device based on the ZnO/ZnS core shell nanowires exhibited a photocurrent approximately 40 times higher than that of the device based on the ZnO nanowires. The differing photoresponse of the detectors was consistent with the existence of surface passivation and localized states. This study provides a means for modifying the optical properties of ZnO materials, and demonstrates the potential of ZnO/ZnS core shell nanowires in UV excitonic emission and detection.
收录类别	SCI ; EI
内容类型	期刊论文
源URL	[http://ir.ciomp.ac.cn/handle/181722/55239]
专题	长春光学精密机械与物理研究所_中科院长春光机所知识产出
推荐引用方式 GB/T 7714	Fang, X.,Z. P. Wei,R. Chen,et al. Influence of Exciton Localization on the Emission and Ultraviolet Photoresponse of ZnO/ZnS Core-Shell Nanowires[J]. Acs Applied Materials & Interfaces,2015,7(19):10331-10336.
APA	Fang, X..,Z. P. Wei.,R. Chen.,J. L. Tang.,H. F. Zhao.,...&X. Y. Chu and X. H. Wang.(2015).Influence of Exciton Localization on the Emission and Ultraviolet Photoresponse of ZnO/ZnS Core-Shell Nanowires.Acs Applied Materials & Interfaces,7(19),10331-10336.
MLA	Fang, X.,et al."Influence of Exciton Localization on the Emission and Ultraviolet Photoresponse of ZnO/ZnS Core-Shell Nanowires".Acs Applied Materials & Interfaces 7.19(2015):10331-10336.

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