Catalytic oxidation of toluene over active MnO (x) catalyst prepared via an alkali-promoted redox precipitation method | |
Wang, Lei1,2; Zhang, Chuanhui2; Huang, He2; Li, Xuebing2; Zhang, Wei1; Lu, Mohong1; Li, Mingshi1 | |
刊名 | REACTION KINETICS MECHANISMS AND CATALYSIS
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2016-08-01 | |
卷号 | 118期号:2页码:605-619 |
关键词 | VOCs MnOx Redox precipitation Reducibility Average oxidation state |
英文摘要 | MnO (x) catalysts were contrastively prepared by an alkali-promoted redox precipitation strategy (MnO (x) -RP) and a conventional citrate sol-gel method (MnO (x) -SG), and tested for the catalytic oxidation of toluene, where MnO (x) -RP exhibited higher catalytic activity, excellent catalytic durability under dry conditions and good regeneration ability under humid conditions. The characterizations results indicated that different crystalline phases but similar textual properties (specific surface area, porosity and morphology) were observed over MnO (x) -RP and MnO (x) -SG catalysts, while MnO (x) -RP presented significantly higher low-temperature reducibility and average oxidation state of Mn as well as higher abundance of surface adsorbed oxygen species compared with MnO (x) -SG, thus beneficially resulting in its superior catalytic activity in the reaction. |
WOS标题词 | Science & Technology ; Physical Sciences |
类目[WOS] | Chemistry, Physical |
研究领域[WOS] | Chemistry |
关键词[WOS] | MANGANESE OXIDE CATALYSTS ; VOLATILE ORGANIC-COMPOUNDS ; ORDERED MACROPOROUS LAMNO3 ; HIGH-EFFICIENCY CATALYSTS ; PEROVSKITE CATALYST ; ROOM-TEMPERATURE ; HIGH-PERFORMANCE ; CARBON-MONOXIDE ; COMBUSTION ; VOCS |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000379345000018 |
内容类型 | 期刊论文 |
源URL | [http://ir.qibebt.ac.cn/handle/337004/8393] ![]() |
专题 | 青岛生物能源与过程研究所_多相催化转化团队 |
作者单位 | 1.Changzhou Univ, Sch Petrochem Engn, Jiangsu Key Lab Adv Catalyt Mat & Technol, Changzhou 213164, Peoples R China 2.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Key Lab Biofuels, Qingdao 266101, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Lei,Zhang, Chuanhui,Huang, He,et al. Catalytic oxidation of toluene over active MnO (x) catalyst prepared via an alkali-promoted redox precipitation method[J]. REACTION KINETICS MECHANISMS AND CATALYSIS,2016,118(2):605-619. |
APA | Wang, Lei.,Zhang, Chuanhui.,Huang, He.,Li, Xuebing.,Zhang, Wei.,...&Li, Mingshi.(2016).Catalytic oxidation of toluene over active MnO (x) catalyst prepared via an alkali-promoted redox precipitation method.REACTION KINETICS MECHANISMS AND CATALYSIS,118(2),605-619. |
MLA | Wang, Lei,et al."Catalytic oxidation of toluene over active MnO (x) catalyst prepared via an alkali-promoted redox precipitation method".REACTION KINETICS MECHANISMS AND CATALYSIS 118.2(2016):605-619. |
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