PdO nanoparticles enhancing the catalytic activity of Pd/carbon nanotubes for 4-nitrophenol reduction | |
Wang, Chunxia1; Yang, Fan2; Yang, Wang2; Ren, Liang2; Zhang, Yunhan2; Jia, Xilai2; Zhang, Liqiang2; Li, Yongfeng2 | |
刊名 | RSC ADVANCES
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2015 | |
卷号 | 5期号:35页码:27526-27532 |
英文摘要 | In this work, we demonstrate that the presence of PdO nanoparticles can significantly enhance the catalytic performance of Pd catalysts for the reduction of 4-nitrophenol (4-NP). Heterogeneous Pd/PdO nanoparticles supported on an oxidized multi-walled carbon nanotube (OCNTs) catalyst is prepared by a one-pot gas-liquid interfacial plasma (GLIP) method with the precursor Pd(NO3)(2)center dot 2H(2)O. The Pd/PdO catalysts with uniform size distribution exhibit remarkable catalytic activity during the reduction of 4-NP to 4-aminophenol (4-AP) in neat water at room temperature. The turnover frequency (TOF) value is up to 750 h(-1), which shows much higher catalytic activity than single Pd nanoparticles supported on OCNTs. Our results indicate that the Pd/PdO catalyst can be readily recovered and reused 10 times. |
收录类别 | SCI |
语种 | 英语 |
公开日期 | 2016-05-09 |
内容类型 | 期刊论文 |
源URL | [http://ir.iccas.ac.cn/handle/121111/28464] ![]() |
专题 | 化学研究所_活体分析化学实验室 |
作者单位 | 1.Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Key Lab Analyt Chem Living Biosyst, Beijing 100190, Peoples R China 2.China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Chunxia,Yang, Fan,Yang, Wang,et al. PdO nanoparticles enhancing the catalytic activity of Pd/carbon nanotubes for 4-nitrophenol reduction[J]. RSC ADVANCES,2015,5(35):27526-27532. |
APA | Wang, Chunxia.,Yang, Fan.,Yang, Wang.,Ren, Liang.,Zhang, Yunhan.,...&Li, Yongfeng.(2015).PdO nanoparticles enhancing the catalytic activity of Pd/carbon nanotubes for 4-nitrophenol reduction.RSC ADVANCES,5(35),27526-27532. |
MLA | Wang, Chunxia,et al."PdO nanoparticles enhancing the catalytic activity of Pd/carbon nanotubes for 4-nitrophenol reduction".RSC ADVANCES 5.35(2015):27526-27532. |
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