Speeding up CFD simulation of fluidized bed reactor for MTO by coupling CRE model | |
Lu, Bona1,2; Luo, Hao1; Li, Hua3; Wang, Wei1; Ye, Mao3; Liu, Zhongmin3; Li, Jinghai1 | |
刊名 | CHEMICAL ENGINEERING SCIENCE |
2016-04-02 | |
卷号 | 143期号:APR页码:341-350 |
关键词 | CRE CFD Methanol-to-olefins (MTO) EMMS Kinetics Fluidized bed |
ISSN号 | 0009-2509 |
通讯作者 | Wang, W (reprint author), Chinese Acad Sci, Inst Proc Engn, Sate Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China. |
英文摘要 | The methanol to olefins (MTO) process opens an economical and important route to produce light olefins. The design of MTO reactor borrows ideas from the reaction-regeneration configuration of the modern fluid catalytic cracking (FCC) units. However, their hydrodynamic behaviors are quite different in the sense that the fluidized bed for MTO reactions operates in different flow regime from that of FCC, calling for new modeling for scale-up. In addition, the coke deposited on catalysts greatly affects the MTO reaction while its generation is very slow. It normally takes tens of minutes or even hours for catalysts to reach the desired level of coke content. Time-dependent computational fluid dynamics (CFD) simulation of such a long process poses a big challenge to reactive multiphase flow modeling. To speed up it, we try to integrate the classic chemical reaction engineering (CRE) model with CFD. In particular, the continuous stirred tank reactor (CSTR) model is established to estimate the steady state distribution of coke content, which is then set as the initial distribution for CFD simulation to shorten the time to reach the steady state of reactive flows. Comparison with experimental data shows good agreement and also great speed-up ratio compared to traditional CFD simulation. (C) 2016 Elsevier Ltd. All rights reserved. |
WOS标题词 | Science & Technology ; Technology |
类目[WOS] | Engineering, Chemical |
研究领域[WOS] | Engineering |
关键词[WOS] | SOLID RISER FLOWS ; TO-OLEFINS PROCESS ; EMMS MODEL ; METHANOL ; HYDRODYNAMICS ; FORMULATION ; MECHANISMS ; BOILER ; EFM |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000371472200030 |
内容类型 | 期刊论文 |
源URL | [http://ir.ipe.ac.cn/handle/122111/20642] |
专题 | 过程工程研究所_研究所(批量导入) |
作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, Sate Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Beijing 10049, Peoples R China 3.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Natl Engn Lab MTO, Dalian 116023, Peoples R China |
推荐引用方式 GB/T 7714 | Lu, Bona,Luo, Hao,Li, Hua,et al. Speeding up CFD simulation of fluidized bed reactor for MTO by coupling CRE model[J]. CHEMICAL ENGINEERING SCIENCE,2016,143(APR):341-350. |
APA | Lu, Bona.,Luo, Hao.,Li, Hua.,Wang, Wei.,Ye, Mao.,...&Li, Jinghai.(2016).Speeding up CFD simulation of fluidized bed reactor for MTO by coupling CRE model.CHEMICAL ENGINEERING SCIENCE,143(APR),341-350. |
MLA | Lu, Bona,et al."Speeding up CFD simulation of fluidized bed reactor for MTO by coupling CRE model".CHEMICAL ENGINEERING SCIENCE 143.APR(2016):341-350. |
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